New nonlinear optical crystal: cesium lithium borate

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Abstract

A new ultraviolet nonlinear crystal, CsLiB6O10 (CLBO), is presented. CLBO can be grown from stoichiometric melt and from solution, and a large crystal with dimensions of 14 × 11 × 11 cm3 was obtained, demonstrating the ability to obtain large crystals with a high growth rate. Fourth- and fifth harmonic generation of Nd:YAG laser radiation at λ = 266 and 213 nm were obtained in CLBO crystals. The crystals are well suited for higher-order harmonic generation because of the sufficient large nonlinear coefficient, large values of angular, spectral, and temperature bandwidths, and small walk-off angles.

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Mori, Y., Kuroda, I., Nakajima, S., Sasaki, T., & Nakai, S. (1995). New nonlinear optical crystal: cesium lithium borate. Applied Physics Letters, 67(13), 1818–1820. https://doi.org/10.1063/1.115413

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