Recent progress in research and development in neutron resonance densitometry (NRD) for quantification of nuclear materials in particle-like debris

Abstract

To quantify special nuclear materials (SNM) in particle-like debris, a technique named neutron resonance densitometry (NRD) has been proposed. This method is a combination of neutron resonance transmission analysis (NRTA) and neutron resonance capture analysis (NRCA) or prompt gamma-ray analysis (PGA). In NRTA, neutron transmission rate is measured as a function of neutron energy with a short flight path time-of-flight (TOF) system. Characteristic neutron transmission dips of Pu and U isotopes are used for their quantification. Materials in the samples (H, B, Cl, Fe, etc.) are measured by the NRCA/PGA method. For the NRD measurements, a compact TOF facility is designed. The statistical uncertainties of the obtained quantities of the SNMs in a sample are estimated. A high-energyresolution and high-S/N γ-ray spectrometer is under development for NRCA/PGA. Experimental studies of systematic uncertainties concerning the sample properties, such as thickness and uniformity, are in progress at the TOF facility GELINA of European Commission (EC), Joint Research Centre (JRC), Institute for Reference Materials and Measurements (IRMM).