Preparation of Honeycomb-Structured Activated Carbon-Zeolite Composites from Modified Fly Ash and the Adsorptive Removal of Pb(II)

Abstract

In this paper, fly ash (FA) was successfully prepared into a honeycomb carbon-zeolite composite (CZC) with good adsorption and used for the removal of Pb(II) by a two-step method. Compared with general FA, the honeycomb structure of the CZC resulted in a ∼6× increase in the specific surface area, and the average pore size increased from 3.4 to 12.7 μm. The maximum adsorption capacity of CZCs for Pb(II) reached 185.68 mg/g in 40 min. The experimental data for the adsorption of Pb(II) by CZC showed that the results were in good agreement with the Langmuir adsorption model. The adsorbent prepared in this study has good application prospects in wastewater treatment and provides a new method for the resource recovery of FA.