Determining the susceptibility of cloud albedo to changes in droplet concentration with the Advanced Very High Resolution Radiometer

Abstract

A calculation of cloud susceptibility, defined in this work as the increase in albedo resulting from the addition of one cloud droplet per cubic centimeter (as cloud liquid water content remains constant), is made through the satellite remote sensing of cloud droplet radius and optical thickness. The remote technique uses spectral channels of the AVHRR instrument on board NOAA polar-orbiting satellites. Radiative transfer calculations of reflectance and effective surface and cloud emissivities are made for applicable sun and satellite viewing angles, including azimuth, at various radii and optical thicknesses for each AVHRR channel. Emission in channel 3 (at 3.75 μm) is removed to give the reflected solar component. These calculations are used to infer the radius and optical thickness that best match the satellite measurements. The retrieved range of susceptibilities for all marine stratus clouds studied varied by about two orders of magnitude. This variation implies that climate studies that include possible marine stratus albedo modification from anthropogenic CCN are incomplete without accounting for existing susceptibilities. -from Authors