Ultrasound-assisted one-pot multi-component synthesis of 2-pyrrolidinon- 3-olates catalyzed by Co3O4@SiO2 core-shell nanocomposite

Abstract

2-pyrrolidinon-3-olates were synthesized via one-pot four-component reaction of 2-aminobenzothiazole, aromatic aldehydes, dimethyl acetylenedicarboxylate and morpholine/ piperidine in the presence of Co3O4@SiO2 core-shell nanocomposite as catalyst under ultrasound irradiation. The protocol offers several such advantages as high yields, short reaction time and mild reaction conditions with reusability of the catalyst. The core-shell nanocomposite was also prepared using ultrasound irradiation and the structure and magnetic properties were fully characterized by TEM, FE-SEM, XRD, EDX, FT-IR and VSM analysis.