Optical signatures of type-II Weyl fermions in the noncentrosymmetric semimetals RAlSi (R=La, Ce, Pr, Nd, Sm)

Abstract

Weyl semimetals with magnetic ordering provide a promising platform for the investigation of rare topological effects such as the anomalous Hall effect, resulting from the interplay of nontrivial bands with various spin configurations. The materials RAlSi, where R represents a rare-earth element, are prominent representatives of Weyl semimetals, where the Weyl states are induced by space inversion symmetry breaking, and in addition, for several rare-earth elements R, enhanced by time-reversal symmetry breaking through the formation of a magnetic order at low temperature. We report optical signatures of Weyl fermions in the magnetic compounds CeAlSi, PrAlSi, NdAlSi, and SmAlSi as well as the nonmagnetic family member LaAlSi by broad-frequency infrared spectroscopy at room temperature, i.e., in the paramagnetic phase. A similar profile of the optical conductivity spectrum and a metallic character are observed for all compounds, with LaAlSi showing the strongest free charge-carrier contribution. Furthermore, the linear-in-frequency behavior of the optical conductivity of all investigated compounds indicates the presence of Weyl nodes in close proximity to the Fermi energy, resulting from inversion symmetry breaking in noncentrosymmetric structures. According to the characteristics of these linear slopes, the RAlSi compounds are expected to host mainly type-II Weyl states with overtilted Weyl cones. The results are compared to the optical response of the closely related RAlGe materials, which are considered as potential hybridization-driven Weyl-Kondo systems.