Effects of annealing conditions on mixed lead halide perovskite solar cells and their thermal stability investigation

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Abstract

In this work, efficient mixed organic cation and mixed halide (MA0.7FA0.3Pb(I0.9Br0.1)3) perovskite solar cells are demonstrated by optimizing annealing conditions. AFM, XRD and PL measurements show that there is a better perovskite film quality for the annealing condition at 100 °C for 30 min. The corresponding device exhibits an optimized PCE of 16.76% with VOC of 1.02 V, JSC of 21.55 mA/cm2 and FF of 76.27%. More importantly, the mixed lead halide perovskite MA0.7FA0.3Pb(I0.9Br0.1)3 can significantly increase the thermal stability of perovskite film. After being heated at 80 °C for 24 h, the PCE of the MA0.7FA0.3Pb(I0.9Br0.1)3 device still remains at 70.00% of its initial value, which is much better than the control MAPbI3 device, where only 46.50% of its initial value could be preserved. We also successfully fabricated high-performance flexible mixed lead halide perovskite solar cells based on PEN substrates.

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Yang, H., Zhang, J., Zhang, C., Chang, J., Lin, Z., Chen, D., … Hao, Y. (2017). Effects of annealing conditions on mixed lead halide perovskite solar cells and their thermal stability investigation. Materials, 10(7). https://doi.org/10.3390/ma10070837

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