Hidden electronic phase in strained few-layer 1 T-TaS2

Abstract

Layered van der Waals materials are exciting as they often host multiple, competing electronic phases. This article reports the experimental observation of the coexistence of insulating and metallic phases deep within the commensurate charge density wave phase in high-quality devices of few-layer 1T-TaS2. Through detailed conductance fluctuation spectroscopy of the electronic ground state, we establish that the mixed phase consists of insulating regions surrounded by one-dimensional metallic domain walls. We show that the electronic ground state of 1T-TaS2 can be affected drastically by strain, eventually leading to the collapse of the Mott gap in the commensurate charge density wave phase. Our study resolves an outstanding question, namely the effect of the interlayer coupling strength on the electronic phases in layered van der Waals materials.