Elucidating charge delocalization in the high-spin state of aqueous Fe II spin-crossover compounds via time-resolved spectroscopy in the x-ray water window

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Abstract

We report the first time-resolved spectroscopy of aqueous solution in the Xray water window. Nitrogen K-edge spectra, combined with ab initio calculations, reveal distinct charge delocalization, shedding light on the origins of ultrafast spin crossover. © Owned by the authors, published by EDP Sciences, 2013.

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Huse, N., Van Kuiken, B. E., Cho, H., Strader, M. L., Kim, T. K., Khalil, M., & Schoenlein, R. W. (2013). Elucidating charge delocalization in the high-spin state of aqueous Fe II spin-crossover compounds via time-resolved spectroscopy in the x-ray water window. In EPJ Web of Conferences (Vol. 41). https://doi.org/10.1051/epjconf/20134105037

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