Spectral dynamics in the B800 band of LH2 from Rhodospirillum molischianum: A single-molecule study

Abstract

The BChl α absorptions in the B800 spectrum of individual LH2 complexes from Rhodospirillum molischianum show sudden, reversible spectral jumps between a finite number of spectral positions. From our data, we conclude that these fluctuations result from conformational changes of the protein backbone in close vicinity of the chromophores which provides a sensitive tool to monitor local modulations of the pigment-protein interaction.