Strong Coupling between a Quasi-single Molecule and a Plasmonic Cavity in the Trapping System

Abstract

We theoretically investigate the strong coupling phenomenon between a quasi-single molecule and a plasmonic cavity based on the blue-detuned trapping system. The trapping system is made up of a metallic nanohole array. A finite-difference time-domain method is employed to simulate the system, and the molecule is treated as a dipole in simulations. By calculating the electromagnetic field distributions, we obtain the best position for trapping a molecule, and we get the strong coupling phenomenon that there are two splitting peaks in the transmission spectrum when the molecule is trapped in the structure, while only one peak is observed in the one without the molecule. We also find that only when the molecule polarization parallels to the incident light wave vector can we observe a strong coupling phenomenon.