Observation of large anomalous Nernst effect in 2D layered materials Fe 3 GeTe 2

Abstract

Two-dimensional layered materials with remarkable thermoelectric coefficients are promising candidates for sustainable thermopower batteries. Here, we investigate the anomalous Nernst effect and anomalous Hall effect in the polycrystalline Fe 3 GeTe 2 thin films. While its Seebeck coefficient and anomalous Hall angle (or magnetization) monotonously increase and decrease with temperature, respectively, the anomalous Nernst coefficient of the Fe 3 GeTe 2 films exhibits a peak value of 0.28 μV K-1 T-1 at 150 K, which is the compromised outcome between the enhanced Seebeck effect and the gradually weakened magnetism with elevating temperature. A noticeable anomalous Nernst effect observed in Fe 3 GeTe 2 sheds light on the low-temperature application of two-dimensional layered materials in spin-caloritronics.