Magnetic domain study in Fe3GaTe2 ferromagnet with strong perpendicular anisotropy using magnetic force microscopy

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Abstract

We investigate the magnetic domain behavior of bulk Fe 3 GaTe 2 , a van der Waals (vdW) ferromagnet characterized by a Curie temperature ( T c ) of 350-380 K and significant perpendicular magnetic anisotropy (PMA). Using magnetic force microscopy, we present the evolution of magnetic domains during cooling from T c to 300 K, and analyze magnetic domain images along the hysteresis loop at 4.2 K. Our observations reveal a strong temperature-dependent domain structure. From room temperature to T c , we observe the coexistence of stripe, bubble, and surface spike domains. In contrast, in the zero-field cooled state at 4.2 K, irregular stripe and enclosed ring domains predominate. The correlation between global and local magnetization suggests that the hysteretic behavior in the magnetization results from the rapid nucleation of a few stripe domains evolving into intricate dendritic patterns, a phenomenon not previously observed in other vdW systems. These findings highlight the delicate balance among interlayer exchange coupling, thermal fluctuations, and PMA in the formation of various domains in a 3D vdW system, where shape anisotropy is minimized.

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Lee, J., Yun, J., Lee, Y., Tak Kang, B., Sung Kim, J., Haberkorn, N., & Kim, J. (2024). Magnetic domain study in Fe3GaTe2 ferromagnet with strong perpendicular anisotropy using magnetic force microscopy. Journal of Applied Physics, 136(12). https://doi.org/10.1063/5.0230813

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