PISTON and CAMP2Ex observations of the fundamental modes of aerosol vertical variability in the Northwest Tropical Pacific and Maritime Continent's Monsoon

Abstract

While most large-scale smoke advection occurs within the free troposphere, Maritime Continent smoke is suspected to be unique in its long-range, near-surface transport. Such a pathway likely creates strong gradients and uncertainties in interpreting satellite and model data on light extinction, air pollution, and cloud condensation nuclei. This paper documents High Spectral Resolution Lidar (HSRL) data from the 2019 ONR PISTON cruise and NASA CAMP2Ex flights that revealed Maritime Continent smoke and pollution transport pathways and heterogeneity around the Marine Atmospheric Boundary Layer (MABL) over thousands of kilometers. Observations showed that 95% of integrated aerosol backscatter occurred below 2500 m altitude. The R/V Sally Ride observed 50th and 84th percentile aerosol backscatter altitudes at ∼600 and ∼1500 m respectively, regardless of aerosol loading. Peak backscatter values occurred within or near the MABL top, diminishing as we approached 2-3 km altitude, but with occasional plumes reaching the melting level at 4800 m. At monsoonal scales, aerosol models largely account for the observed directional wind shear that causes altitude-dependent particle transport: near-surface particles remain in the core monsoon flow around the MABL, while at lower latitudes, aerosol layers aloft advect more eastwardly. Around the MABL, however, significant cloud-scale variability exists due to fine-scale flow, halo-entrainment-detrainment, and cold pool phenomena. Backscatter enhancements beneath individual clouds, extending to the ocean surface, likely relate to MABL-free troposphere exchange and air-sea interaction. So while aerosol transport occurs near the surface, particle extinction heterogeneity must still be considered for in situ observations and satellite retrievals.