Angle-resolved high-order harmonics in wurtzite-type ZnO

Abstract

High-order harmonics in solids provide a method of analyzing the intraband and interband dynamics of a solid driven by an ultrafast laser. This study analyzed the contributions of intraband and interband dynamics based on angle-resolved high-order harmonics. According to the simulations and experiments, we found that the angular divergences of the harmonics have an evident boundary at the bandgap when the laser is polarized along the asymmetric direction, which is primarily invoked by the interplay of an interband transition and an intraband electron movement, and the intraband and interband dynamics have different sensitivities of the spatial phase of driving laser.