Spin to charge conversion in chemically deposited epitaxial La0.9MnO3 thin films capped with Pt

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Abstract

Spin to charge conversion process in a broad range of temperatures is studied in La0.92MnO3/Pt bilayers prepared by polymer-assisted deposition (PAD). It is shown that an excellent LMO/Pt interface can be obtained in spite of using ex situ deposition of the Pt layer. The values obtained for the effective spin-mixing conductance, g↑↓eff = 0.76 × 1015 cm−2, suggest that significant spin transport across the LMO/Pt interface could be achieved. Spin pumping experiments generate a transversal voltage signal VISHE, due to spin to charge conversion via inverse spin Hall effect, that has been detected down to about 100 K with values of the spin-Hall angle, θSH, of about 2.5%, slightly decreasing on reducing temperature in the analyzed temperature range. These results indicate that LMO is a promising perovskite building block for all-oxide multifunctional high-frequency spintronics devices and that PAD technique provides oxide epitaxial thin films of good quality adequate for spintronic applications.

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Martin-Rio, S., Pomar, A., Frontera, C., Wang, H., Manzorro, R., Magén, C., … Martinez, B. (2022). Spin to charge conversion in chemically deposited epitaxial La0.9MnO3 thin films capped with Pt. Journal of Materials Chemistry C, 10(15), 5914–5921. https://doi.org/10.1039/d2tc00048b

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