Unusual evolution of Bc 2 and T c with inclined fields in restacked TaS2 nanosheets

Abstract

Recently we reported an enhanced superconductivity in restacked monolayer TaS2 nanosheets compared with the bulk TaS2, pointing to the exotic physical properties of low dimensional systems. Here we tune the superconducting properties of this system with magnetic field along different directions, where a strong Pauli paramagnetic spin-splitting effect is found in this system. Importantly, an unusual enhancement as high as 3.8 times of the upper critical field B c2, as compered with the Ginzburg-Landau (GL) model and Tinkham model, is observed under the inclined external magnetic field. Moreover, with the out-of-plane field fixed, we find that the superconducting transition temperature T c can be enhanced by increasing the in-plane field and forms a dome-shaped phase diagram. An extended GL model considering the special microstructure with wrinkles was proposed to describe the results. The restacked crystal structure without inversion center along with the strong spin-orbit coupling may also play an important role for our observations.