Two-dimensional gradients in magnetic properties created with direct-write laser annealing

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Abstract

Across the fields of magnetism, microelectronics, optics, and others, engineered local variations in material properties can yield groundbreaking functionalities that play a crucial role in enabling future technologies. One-dimensional lateral gradients in material properties give rise to a plethora of new effects in thin-film magnetic systems. However, extending such gradient-induced behaviors to two dimensions has been challenging to realize experimentally. Here, we demonstrate the creation of two-dimensional complex patterns with continuous variations in magnetic anisotropy, interlayer exchange coupling, and ferrimagnetic compensation at the mesoscopic scale in numerous application-relevant magnetic materials. We exploit our engineered gradients in material properties to demonstrate novel magnetic functionalities, including the creation of a spin wave band pass filter and an architecture for passively resetting the position of a magnetic domain wall. Our results highlight the exciting new physics and device applications enabled by two-dimensional gradients in thin film properties.

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Riddiford, L. J., Brock, J. A., Murawska, K., Wisser, J., Huang, X., Shepelin, N. A., … Heyderman, L. J. (2025). Two-dimensional gradients in magnetic properties created with direct-write laser annealing. Nature Communications , 16(1). https://doi.org/10.1038/s41467-025-65921-7

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