Enviro-HIRLAM model estimates of elevated black carbon pollution over Ukraine resulted from forest fires

Abstract

Biomass burning is one of the biggest sources of atmospheric black carbon (BC), which negatively impacts human health and contributes to climate forcing. In this work, we explore the horizontal and vertical variability of BC concentrations over Ukraine during wildfires in August 2010. Using the Enviro-HIRLAM modelling framework, the BC atmospheric transport was modelled for coarse, accumulation, and Aitken mode aerosol particles emitted by the wildfire. Elevated pollution levels were observed within the boundary layer. The influence of the BC emissions from the wildfire was identified up to 550hPa level for the coarse and accumulation modes and at distances of about 2000km from the fire areas. BC was mainly transported in the lowest 3km layer and mainly deposited at night and in the morning hours due to the formation of strong surface temperature inversions. As modelling is the only available source of BC data in Ukraine, our results were compared with ground-level measurements of dust, which showed an increase in concentration of up to 73% during wildfires in comparison to average values. The BC contribution was found to be 10%-20% of the total aerosol mass near the wildfires in the lowest 2km layer. At a distance, BC contribution exceeded 10% only in urban areas. In the areas with a high BC content represented by both accumulation and coarse modes, downwelling surface long-wave radiation increased up to 20Wm-2, and 2m air temperature increased by 1-4°C during the midday hours. The findings of this case study can help to understand the behaviour of BC distribution and possible direct aerosol effects during anticyclonic conditions, which are often observed in mid-latitudes in the summer and lead to wildfire occurrences.