Development of a flex and stretchy conductive cotton fabric via flat screen printing of PEDOT:PSS/PDMS conductive polymer composite

Abstract

In this work, we have successfully produced a conductive and stretchable knitted cotton fabric by screen printing of poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS) and poly(dimethylsiloxane-b-ethylene oxide)(PDMS-b-PEO) conductive polymer composite. It was observed that the mechanical and electrical properties highly depend on the proportion of the polymers, which opens a new window to produce PEDOT:PSS-based conductive fabric with distinctive properties for different application areas. The bending length analysis proved that the flexural rigidity was lower with higher PDMS-b-PEO to PEDOT:PSS ratio while tensile strength was increased. The SEM test showed that the smoothness of the fabric was better when PDMS-b-PEO is added compared to PEDOT:PSS alone. Fabrics with electrical resistance from 24.8 to 90.8 kΩ/sq have been obtained by varying the PDMS-b-PEO to PEDOT:PSS ratio. Moreover, the resistance increased with extension and washing. However, the change in surface resistance drops linearly at higher PDMS-b-PEO to PEDOT:PSS ratio. The conductive fabrics were used to construct textile-based strain, moisture and biopotential sensors depending upon their respective surface resistance.