Enhancement in the critical current density of BaTiO3-doped YBCO films by low-energy (60 keV) proton irradiation

Abstract

Although YBa2Cu3O72212δ (YBCO) is one of the most promising superconducting materials for power applications, the fabrication of low-cost coated conductors with the high in-field performance remains challenging. Here, we report an efficient mixed-pinning landscape for enhancing the in-field performance of BaTiO3 (BTO)-doped YBCO films by low-energy (60 keV) proton irradiation. The smaller (2-4 nm), weaker but perhaps denser pinning sites have been successfully introduced by irradiation, which can form a mixed-pinning landscape with pre-doped BTO precipitates (5-15 nm), leading to the increased vortex pinning. In this case, the critical current density (J c) of YBCO films increases significantly, especially at low temperature and high magnetic field, and it increases three times near 6 T at 20 K when the irradiation dose is 1 × 1015 proton cm-2. Additionally, the c-axis length (c-parameter) of YBCO increases with the increase of irradiation dose, which indicates the decreasing oxygen content due to the excessive irradiation, thereby the reduction in critical transition temperature (T c). Employing low irradiation energy is beneficial for protons to stop inside YBCO film and thereby induces higher density defects when applying low doses. This fabrication technique is a practicable post-production solution to improve the in-field performance of nanoparticle-doped YBCO films.