A typical weather pattern for ozone pollution events in North China

Abstract

Ground-level observations, reanalyzed meteorological fields and a 3-D global chemical and transport model (GEOS-Chem) were applied in this study to investigate ozone ( O3) pollution events (OPEs) in North China (36.5-40.5 ĝ N, 114.5-119.5 ĝ E) during 2014-2017. Ozone pollution days (OPDs) were defined as days with maximum daily averaged 8 h (MDA8) concentrations over North China larger than 160 μ g m -3, and OPEs were defined as periods with 3 or more consecutive OPDs. Observations showed that there were 167 OPDs and 27 OPEs in North China during 2014-2017, in which 123 OPDs and 21 OPEs occurred from May to July. We found that OPEs in North China occurred under a typical weather pattern with high daily maximum temperature (Tmax), low relative humidity (RH), anomalous southerlies and divergence in the lower troposphere, an anomalous high-pressure system at 500 hPa, and an anomalous downward air flow from 500 hPa to the surface. Under such a weather pattern, chemical production of O3 was high between 800 and 900 hPa, which was then transported downward to enhance O3 pollution at the surface. A standardized index I-OPE was defined by applying four key meteorological parameters, including Tmax, RH, meridional winds at 850 hPa (V850) and zonal winds at 500 hPa (U500). I-OPE can capture approximately 80 % of the observed OPDs and OPEs, which has implications for forecasting OPEs in North China..