Performance-tuning of PVA-based gel electrolytes by acid/PVA ratio and PVA molecular weight

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Abstract

The significant breakthroughs of flexible gel electrolytes have attracted extensive attention in modern wearable electronic gadgets. The lack of all-around high-performing gels limits the advantages of such devices for practical applications. To this end, developing a multi-functional gel architecture with superior ionic conductivity while enjoying good mechanical flexibility is a bottleneck to overcome. Herein, an architecturally engineered gel, based on PVA and H3PO4 with different molecular weights of PVA for various PVA/H3PO4 ratios, was developed. The results show the dependence of ionic conductivity on molecular weight and also charge carrier concentration. Consequently, fine-tuning of PVA-based gels through a simple yet systematic and well-regulated strategy to achieve highly ion-conducting gels, with the highest ionic conductivity of 14.75 ± 1.39 mS cm-1 have been made to fulfill the requirement of flexible devices. More importantly, gel electrolytes possess good mechanical robustness while exhibiting high-elasticity (%766.66 ± 59.73), making it an appropriate candidate for flexible devices.

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Alipoori, S., Torkzadeh, M. M., Mazinani, S., Aboutalebi, S. H., & Sharif, F. (2021). Performance-tuning of PVA-based gel electrolytes by acid/PVA ratio and PVA molecular weight. SN Applied Sciences, 3(3). https://doi.org/10.1007/s42452-021-04182-7

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