Temperature dependence of magnetization at zero applied magnetic field in nearly two dimensional ferromagnets

Abstract

NMR measurement have been made at low temperatures on the crystal structure of K2CuF4 and (C3H7NH 3)2CuCl4 at zero applied magnetic field. 63Cu, 65Cu and 35Cl NMR have been used to measure spontaneous magnetization at the temperature range 2 K down to 30 mK. We have made the NMR experiments using a 3He-4He dilution refrigerator by conventional pulsed NMR method without external magnetic field. The magnetization at zero applied magnetic field in the nearly two-dimensional ferromagnet K2CuF4 of the experimental data is in a good agreement with Yamaji-Kondo theory and θC = 0.3, which is applied the double-time Green's function method incorporated with Tyablikov's decoupling. For temperature 1.1 K down to 0.26 K, the spontaneous magnetization of (C3H7NH3)2CuCl4 is support (t log t')-formalism from the spin wave theory.